When you no longer need your Enterprise on-premise content connected to the cloud,
you can remove the sync.
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Hover over a synced file/folder in the library and click More
then Unsync from Cloud.
Tip: Files and folders synced to the cloud display the
icon. Contents of a folder
that have been synced display the 
icon.You must unsync the content at the same location where you applied the sync. This means that to unsync a file that was synchronized with its parent folder, you must unsync that parent folder.
Tip: Click so view the location of the parent folder.You're prompted to confirm the sync removal and you can either leave a copy of the synced content in SkyVault Share in the Cloud or delete it. Select the Remove from the cloud option to remove the content from the cloud.
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Click Remove sync.
The cloud icon to the left of the content is cleared, indicating the sync has been removed.